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The maximum Tc of conventional superconductors at ambient pressure
Authors: Kun Gao, Tiago F.T. Cerqueira, Antonio Sanna, Yue-Wen Fang, Đorđe Dangić, Ion Errea, Hai-Chen Wang, Silvana Botti, Miguel A.L. Marques
Ref.: Nat. Commun. 16(1), 8253 (2025)
Abstract: The theoretical maximum critical temperature (Tc) for conventional superconductors at ambient pressure remains a fundamental question in condensed matter physics. Through analysis of electron-phonon calculations for over 20,000 metals, we critically examine this question. We find that while hydride metals can exhibit maximum phonon frequencies of more than 5000 K, the crucial logarithmic average frequency omega log\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${\omega }_{\log }$$\end{document} rarely exceeds 1800 K. Our data reveals an inherent trade-off between omega log\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$${\omega }_{\log }$$\end{document} and the electron-phonon coupling constant lambda, suggesting that the optimal Eliashberg function that maximizes Tc is unphysical. Based on our calculations, we identify Li2AgH6 and its sibling Li2AuH6 as theoretical materials that likely approach the practical limit for conventional superconductivity at ambient pressure. Analysis of thermodynamic stability indicates that compounds with higher predicted Tc values are increasingly unstable, making their synthesis challenging. While fundamental physical laws do not strictly limit Tc to low-temperatures, our analysis suggests that achieving room-temperature conventional superconductivity at ambient pressure is extremely unlikely.
